地球科学进展 ›› 1999, Vol. 14 ›› Issue (1): 37 -43. doi: 10.11867/j.issn.1001-8166.1999.01.0037

全球变化研究 上一篇    下一篇

臭氧变化及其气候效应的研究进展
王体健 1,孙照渤 2   
  1. 1.南京大学大气科学系 南京 210093;2.南京气象学院 南京 210044
  • 收稿日期:1998-04-10 修回日期:1998-08-10 出版日期:1999-02-01
  • 通讯作者: 王体健,男,1968年10月出生,讲师,主要从事区域酸沉降的数值模拟、大气化学和气候相互作用等方面的研究。

DEVELOPMENT OF STUDY ON OZONE VARIATION AND ITS CLIMATIC EFFECT

WANG Tijian 1,SUN Zhaob 2
  

  1. 1.Department of Atmospheric Science,Nanjing University,Nanjing210093;2.Nanjing Institute of Meteorology,Nanjing 210044
  • Received:1998-04-10 Revised:1998-08-10 Online:1999-02-01 Published:1999-02-01

综述了近20年来臭氧变化的规律和机制及其气候效应等领域的研究进展,指出对流层臭氧(主要在北半球)增加、平流层臭氧减少和臭氧总量减少是全球臭氧的变化趋势,原因主要是人类活动导致的NOx、NMHC、CO、CH4等对流层臭氧前体物的增加和NOx、H2O、N2O、CFCs等平流层臭氧损耗物质的增加。臭氧变化引起的气候效应表现在对流层臭氧的增加将带来地表和低层大气的升温,平流层臭氧的减少则可能导致地表和低层大气的升温或降温。将全球或区域气候模式和大气化学模式进行完全耦合来研究臭氧变化的气候效应是一种十分有效的手段,具有广阔的应用前景。

In this paper,the developments of study on characteristics and mechanism of ozone variation and its climate effect are reviewed.The amount of tropospheric O3(in NorthHemisphere)is increasing,that of stratospheric O3is decreasing and the total ozone amount also is decreasing which show the trend of global ozone variation.The main reason is that the O3precusors,such as NOx,NMHC,CO,CH4,are increasing due to human activities and the species(NOx,H2O,N2O,CFCs)which can destroy stratospheric O3are increasing.The enhancement of tropospheric O3will warm the ground surface and the lower atmosphere and the depletion of stratospheric O3may warm or cool the ground surface and lower atmosphere.It is a very effective way to use the global or regional climate model coupled with a atmospheric chemistry model for study on ozone variation and its climate effect.

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1 WMO.Scientific assessment of ozone depletion:Chapter 21.Preprint December 17,1991.
2 IPCC.Climate Change 1994:Radiative forcing of climate change and an evaluation of the IPCC IS92 emission scenarios.In:Houghton J T,Meira Filho L G,Bruce JHoesung Lee,et al,eds.WMO/UNEP,Cambridge University Press,UK 1995.
3 WMO.Scientific assessment of ozone depletion 1994:Global ozone research and monitoring project report No37.World Meteorological Organisation,Geneva.1994.
4 McCormick M P,Veiga R E,Chu W P.Stratospheric ozone profile and total ozone trends derived from the SAGEⅠand SAGEⅡdata.Geophys Res Lett,1992,19:269~272.
5 Stolarski R S,Bloomfield P,McPeters R D,et al.Total ozone trends deduced from Nimbus 7 TOMS data.Geophys Res Lett,1991,18:1015~1018.
6 Logan J A.Tropospheric ozone-seasonal behaviour,trends and anthropogenic influence.J Geophys Res,1985,90:10463~10482.
7 尹荣楼,王玮,尹斌.全球温室效应及其影响.北京:文津出版社,1993,149~154.
8 Rumen D,Bojkov.Trends in tropospheric ozone concentration,Atmospheric ozone.Proceedings of the quadrennial ozone symposium held in Halkidiki,Greece.3-7 September 1984,775~781.
9 曲绍厚.全球大气臭氧层的主要特征和变化趋势.地球科学进展,1994,9(5):39~47.
10 魏鼎文,赵延亮,秦芳,等.中国北京和昆明地区大气臭氧层的异常变化.科学通报,1994,39(16):1509~1511.
11 周秀骥.中国地区臭氧总量变化与青藏高原低值中心.科学通报,1995,40(15):1396~1398.
12 Fishman J,Seiler W.Correlative nature of ozone and carbon monoxide in the troposphere:implications for the tropospheric ozone budget.J Geophys Res,1983,88(C6):3662.
13 Luo Chao,Zhou Xiuji.A regional model study of the variations and distributions of ozone and its precursors on eastern asia and west pacific ocean regions.Acta Meteorologica Sinica,1994,8(2):195~202.
14 S A Mckeen,Hsie E Y,Liu S C.A study of the dependence of rural ozone precursors in the Eastern United States. J Geophys Res,1991,96(D6):15377~15394.
15 Jan E Jonson,Ivar S A,Isaksen.Tropospheric ozone chemistry,The impact of cloud chemistry.J Atmos Chem,1993,16(2):99~122.
16 Jinyou Liang,Daniel J Jacob.Effects of aqueous phase cloud chemistry on tropospheric ozone.J Geophys Res,1997,102(D5):5993~6001.
17 WMO/UNEP. The impact on climate of ozone change and aerosols,1993.
18 Solomon S.The mystery of the Antarctic ozone hole.Rev Geophys,1988,26:131~148.
19 Rowland F S,Sato H,Khwaja H,Elliott.The hydrolysis of chlorine nitrate and its possible atmospheric significant. J Phys Chem,1986,90:1985~1988.
20 Jones P D,Wigley T M L.Global and hemispheric temperature anomalies:land and marine instrumental records.In:Boden T A,et aleds. TREND 93: A compendium of data on global change.ORNL/CDLAC-65, Oakridge: Oakridge National Lab, Tenn,USA,1994.603~608.
21 IPCC.Climate Change:the IPCC scientific assessment.Cambridge:Cambridge University Press,1990.365.
22 石广玉.大气臭氧与气溶胶垂直分布的高空气球观测.大气科学,1996,20(4):401~406.
23 Wang W C,Pinto G,Yung Y L.Climatic effects due to halogenated compounds in the earth s atmosphere.J Atmos Sci,1980,37:333~338.
24 Shi Guangyu,Fan Xiaobiao.Chimate-chemical interactions and greenhouse effects of trace gases.Proceedings of the quadrennial ozone symposium held in Charlottesville,Virginia,USA,June,1992.4~13.
25 WMO global ozone research and monitoring project report.1984,(15):32~35.
26 Ashok Sinha,Ralf Toumi.Troposheric ozone,lightning,and climate change.J Geophys Res,1997,102(D9):10667~10672.
27 石广玉.大气微量气体的辐射强迫与温室气候效应.中国科学(B辑),1991,7:776~784.
28 Ramanathan V, Calls L B, Boughner R E.Sensitivity of surface temperature and atmospheric temperature to pertubations in the stratospheric concentrations of ozone and nitrogen dioxide.J Atmos Sci,1976,33:1092~1112.
29 Fels S B,Mahlman J D,Schwarzkopf M D,et al.Stratospheric sensitivity to perturbation in ozone and carbon dioxide:radiative and dynamical response.J Atmos Sci,1980,37:2265~2297.
30 刘健.微量气体气候效应的数值模拟.气象科学,1992,12(3):310~319.
31 钱永甫.臭氧对海平面纬带年平均温度影响的数值模拟.南京大学学报,1994,30(3):534~540.
32 Robert M Mackay,Malcolm K W Ko,Run-Lie Shia,et al.An estimation of the climatic effects of stratospheric ozone losses during the 1980s.Journal of Climate,1997,10:774~788.
33 Boughner R E.The effect of increased carbon dioxide concentration on stratospheric ozone.J Geophys Res,1978,83:1326~1332.
34 Ramanathan V, Cicerone R J, Singh H B.Trace gas trends and their potential role in climate change.J Geophys,1978,Res,1985,90(D3):5547~5566.
35 Lacis A, Wuebbles D, Logan J.Radiative forcing of climate by changes in the vertical distribution of ozone.J Geophys Res,1990,95:9971~9981.
36 樊小标,石广玉.微量气体—气候问题的一维模式研究.气侯变化规律及其数值模拟研究论文集(第二集).北京:气象出版社,1996.11~16.
37 Ko Malcolm K W,Nien Dak Sze,Mikhail Li Vshits,et al.The seasonal and latitudinal behavior of trace gases and O3as simulated by a two-dimensional model of the atmosphere.J Atmos Sci,1984,41:2381.
38 Hough A M.Development of a two-dimensional global troposheric model:Model chemmistry.J Geophys Res,1991,96:7325~7362.
39 Chien Wang,Ronald G Prinn,Andrei Sokolov.A global interactive chemistry and climate model:Formulation and testing.J Geophys Res,1998,103(D3):3399~3417.
40 Liu Yu,Li Weiliang,Zhou Xiuji.Development of the 2-D coupled stratospheric tropospheric dynamical-chemical model-part I:the description of the model and its preliminary results of the model.Acta Meteorologica Sinica,1997,11(3):271~286.
41 刘煜,李维亮,周秀骥.二维全球平流层—对流层动力、辐射和光化学耦合模式的研究Ⅲ:对流层臭氧的收支.中国地区大气臭氧变化及其对气候环境的影响(二).北京:气象出版社,1997.245~256.
42 樊小标,石广玉.大气微量气体和臭氧变化的二维模式的研究.中国地区大气臭氧变化及其对气候环境的影响(二).北京:气象出版社,1997.207~213.
43 Michael P Dudek,Wei-Chyung Wang,Xin-Zhong Liang,et al.A general circulation model study of the climatic effect of observed stratospheric ozone depletion between 1980 and 1990.Proceedings of the quadrennial ozone symposium held in Charlottesville,Virginia,USA,June,1992. 4~13.
44 Rasch P J,Boville B A,Brasseur G P.A three-dimensional general circulation model with coupled chemistry for middle atmosphere.J Geophys Res,1995,100(D5):9041~9071.
45 John Austin.Sensitivity of ozone and temperature to vertical resolution in a GCM with coupled stratospheric chemistry.Q J R Meteorol Soc,1997,123:1405~1431.
46 何东阳,黄美元.我国对流层大气臭氧的数值模拟.大气科学,1993,17(6):741~749.
47 王喜红,李兴生.中国地区对流层臭氧变化和分布的数值研究.气象学报,1998,56(3):333~348.

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