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  • Kunpeng ZANG, Xiaolong SHEN, Kangxuan WEI, Jun WEN, Fengmei PAN, Honghui XU, Yujun JIANG
    Advances in Earth Science. 2024, 39(7): 717-725. https://doi.org/10.11867/j.issn.1001-8166.2024.035

    Based on the reanalysis of ship-borne continuous data observed in 2012 and 2014 and “bottom-up” and “top-down” approaches, the combustion efficiency and CH4 emission rate of flaring equipped on oil and gas platforms in the Penglai Region of the Bohai Sea were studied. The results showed that peak atmospheric CO2 and CH4 mixing ratios of approximately (11~20)×10-6 and (100~260)×10-9 were observed in the downwind area of flaring. The calculated combustion efficiency of associated gas flaring was (97.8±1.1)%, which was better than that in most countries worldwide. The CH4 emission rates of flaring equipped on the oil and gas platforms were 3.6~6.1 Gg/a and 1.80~2.68 Gg/a, estimated using the “bottom-up” and “top-down” approaches, respectively, indicating that the flaring was the primary source of atmospheric CH4. On the other hand, the difference in the results estimated by the “bottom-up” and “top-down” approaches was still remarkable, mostly due to the limited spatiotemporal representation of emission factors and observation data. This study is beneficial for promoting the recycling and reuse of associated gas and reducing CH4 emissions from marine oil and gas exploitation in China.

  • Lingyi LEI, Feipeng WANG, Kunpeng ZANG, Xiaolong LÜ, Zhi ZHANG, Liyang YANG, Jingli MU
    Advances in Earth Science. 2024, 39(11): 1156-1168. https://doi.org/10.11867/j.issn.1001-8166.2024.088

    Evaluating the distribution and sea-air fluxes of dissolved methane (CH4) in mariculture areas is important for understanding how aquaculture contributes to regional CH4 emissions into the atmosphere. Seasonal field surveys conducted in 2023 were used to analyze the temporal and spatial variation of CH4 concentrations in surface water and CH4 air-sea flux in a typical aquaculture system in Sansha Bay, Fujian Province. The results showed that dissolved CH4 concentrations ranged from 9.91 to 609.22 nmol/L, with corresponding air-sea fluxes between 3.46 to 1 188.15 μmol/ (m2·d). Temporally, the CH4 air-sea fluxes were higher in summer and autumn compared to spring and winter. Spatially, CH4 concentrations and air-sea fluxes decreased consistently from the estuary to the bay mouth, with the highest values in the estuarine aquaculture area and the lowest in the bay mouth aquaculture area. Correlation analysis showed that aquacultural activities and terrestrial runoff inputs contributed to the spatiotemporal distribution of CH4 concentrations within the bay. In the macroalgae cultivation zones, CH4 production and emissions during farming periods were significantly lower than during non-farming periods. Additionally, the residual feed and feces generated by fish in cages may result in increased CH4 emissions. Notably, CH4 emissions peaked in summer, due to enhanced aquaculture activities and runoff inputs during the wet season. Future work should focus on investigating CH4 air-sea fluxes in mariculture areas to provide scientific support for CH4 control and emission reduction in aquaculture.