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Advances in Earth Science  2006, Vol. 21 Issue (4): 352-360    DOI: 10.11867/j.issn.1001-8166.2006.04.0352
Articles     
Progress of Black Carbon Aerosol Research I:Emission, Removal and Concentration
Xu Li1,Wang Yaqiang2,Chen Zhenlin3,Luo Yong1,Ren Wanhui4
1.Laboratory for Climate Studies, China Meteorological Administration, Beijing 100081, China; 2.Centre for Atmosphere Watch and Services, Chinese Academy of Meteorological Sciences, Beijing 100081,China;3.China Meteorological Administration, Beijing 100081,China;4.Shenyang Environment Monitoring Center, Shenyang 110016, China
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Abstract  

Black carbon (BC) aerosol recently is a very active research topic, because it has similar effect to global climate warming with green house gases due to its ability of absorbing solar and atmospheric radiation. The emission and concentration of BC aerosol in China are higher than those in other regions of the same latitude. Therefore,more attention has been paid to the BC aerosol in China by scientists than in other countries. The recent progress of BC aerosol research is presented in the two review papers due to length limitation. The emission, removal and concentration of BC aerosol are described in this paper, and the climate effect and developing research domain are discussed in our companion paper. The emission amount of China in 2000 was 1 050 Gg, which is lower than 1 342Gg in 1995. The reduction in BC emission can be resulted partly due to energy change, including larger use of gas rather than raw coal. The atmospheric concentration of BC in cities was a little higher than in the cities overseas, such as in Beijing (3.3~25.6 μg/m3), Xian (0.5~101.3 μg/m3), etc. The BC concentration in the sediments from the South China Sea is also shown. In the present paper, we compare and analyze the emission and concentration of BC among China and other regions of the world, and the uncertainty in BC aerosol research is also discussed.

Key words:  Black carbon aerosol      Emission      Cleanup      Concentration.     
Received:  26 September 2005      Published:  15 April 2006
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CHEN Zhen-lin
XU Li
REN Wan-hui4
WANG Ya-qiang
LUO Yong

Cite this article: 

Xu Li,Wang Yaqiang,Chen Zhenlin,Luo Yong,Ren Wanhui. Progress of Black Carbon Aerosol Research I:Emission, Removal and Concentration. Advances in Earth Science, 2006, 21(4): 352-360.

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http://www.adearth.ac.cn/EN/10.11867/j.issn.1001-8166.2006.04.0352     OR     http://www.adearth.ac.cn/EN/Y2006/V21/I4/352

[1] IPCC. Third Assessment Report, Climate Change 2001: The Scientific Basis[R]. New York: Cambridge University Press,2001.

[2] Xu Li, Okada K, Zhang Peng, et al. An observational study of physical and chemical haracteristics of atmospheric aerosol particles from late Spring to early Autumn over the Beijing area[J]. Chinese Journal of Atmospheric Sciences, 2002,26(3):401-411.[许黎,冈田菊夫,张鹏,.北京地区春末秋初气溶胶理化特性的观测研究[J]. 大气科学, 2002, 26(3):401-411.]

[3] Smith D M, Griffin J J, Goldberg E D. Elemental carbon in marine sediments: A baseline for burning[J]. Nature,1973, 241: 268-270.

[4] Masiello C A,Druffel E R M. Black carbon in deep-sea sediments[J]. Science,1998,280:1 911-1 913.

[5] Zhang Lisheng. The Simulation and Estimation of the Radiation Effects of Sulfate and Soot Aerosol[D]. Beijing: Institute of Atmospheric Physics, Chinese Academy of Sciences, 1999.[张立盛. 硫酸盐和烟尘气溶胶辐射强迫的模拟和估算[D]. 北京: 中国科学院大气物理研究所, 1999.]

[6] Derwent R G, Ryall D B, Jennings S G, et al. Black carbon aerosol and carbon monoxide in European regional polluted air mass at Mace Head, Ireland during 1995-1998[J]. Atmospheric Environment, 2001, 35: 6 371-6 378.

[7] Novakov T, Hansen J E. Black carbon emissions in the United Kingdom during the past four decades: An empirical analysis[J]. Atmospheric Environment,2004, 38: 4 155-4 163.

[8] Reddy M S,Venkataraman C. Inventory of aerosol and sulphur dioxide emissions from India:- Fossil fuel combustion[J]. Atmospheric Environment,2002, 36: 677-697.

[9] Reddy M S,Venkataraman C. Inventory of aerosol and sulphur dioxide emissions from India:- Biomass combustion[J]. Atmospheric Environment,2002, 36: 699-712.

[10] Streets D G, Gupta S, Waldhoff S T, et al. Black carbon emissions in China[J]. Atmospheric Environment,2001,35: 4 281-4 296.

[11] Streets D G, Bond T C, Carmichael G R, et al. An inventory of gaseous and primary aerosol emissions Asia in the year 2000[J]. Journal of Geophysical Research,2003, 108(D21):8 809.

[12] Wu Jian, Fu Congbin. Simulation research of distribution transportation and radiative effects of black carbon aerosol in recent five spring season over East Asia region[J]. Chinese Journal of Atmospheric Sciences,2005, 29(1):111-119.[吴涧,符淙斌. 近五年来东亚春季黑碳气溶胶分布输送和辐射效应的模拟研究[J]. 大气科学,2005, 29(1): 111-119.]

[13] Kasten F. Falling speed of aerosol particles[J]. Journal of Applied Meteorology, 1968, 7: 944-947.

[14] Junge C E.Air Chemistry and Radioactivity[M]. New York: Academic Press, 1963.

[15] Wen Yupu, Xu Xiaobin, Tang Jie, et al. Element characteristics and sources of the atmospheric aerosol in Waliguan, Qinghai province[J]. Journal of Applied Meteorological Science,2001,12(4):400-408.[温玉璞, 徐晓斌, 汤洁,.青海瓦里关大气气溶胶元素富集特征及其来源[J]. 应用气象学报, 2001, 12(4): 400-408.]

[16] Hopper J F, Worthy D E J, Barrie L A, et al. Atmospheric observations of aerosol black carbon, carbon-dioxide, and methane in the high Arctic[J]. Atmospheric Environment,1994,28:3 047-3 054.

[17] Heintzenberg J, Bigg E K. Tropospheric transport of trace substances in the Southern hemisphere[J]. Tellus, 1990, 42B: 355-363.

[18] Kleefeld S, Hoffer A, Krivácsy Z, et al. Importance of organic and blackcarbon in atmospheric aerosols at Mace Head, on the West Coast of Ireland (531190N, 91540W)[J]. Atmospheric Environment, 2002, 36: 4 479-4 490.

[19] Hansen A D A, Lowenthal D H, Chow J C, et al. Black carbon aerosol at McMurdo station, Antarctica[J]. Journal of Air and Waste Management Association, 2001, 51(4): 593-600.

[20] Tang Jie, Wen Yupu, Zhou Lingxi. Observation research of the black carbon aerosol in clean atmosphere regions of western China[J]. Journal of Applied Meteorological Science, 1999, 10(2): 160-169.[汤洁, 温玉璞, 周凌唏. 中国西部大气清洁地区黑碳气溶胶的观测研究[J]. 应用气象学报, 1999, 10(2): 160-169.]

[21] Moloi K, Chimidza S, Lindgren E S, et al. Black carbon, mass and elemental measurements of airborne particles in the village of Serowe, Botswana[J]. Atmospheric Environment,2002, 36:2 447-2 457.

[22] Wang Gengchen, Kong Qinxin, Ren Lixin, et al. Black carbon aerosol and its variations in the urban atmosphere in Beijing area[J].The Chinese Journal of Process Engineering, 2002, 2(suppl.): 284-288.[王庚辰, 孔琴心, 任丽新,.北京地区大气中的黑碳气溶胶及其变化[J]. 过程工程学报, 2002, 2(增刊): 284-288.]

[23] Kim Y P, Moon K C, Lee J H. Organic and elemental carbon in the fine particles at Kosan, Korea[J]. Atmospheric Environment, 2000, 34: 3 309-3 317.

[24] Su Weihan, Zhang Qiupeng, Song Wenzhi, et al. Atmospheric soot aerosol research in coal-burning areas[J]. Environmental Chemistry,1985, 4(special issue): 134-136.[苏维翰, 张秋彭, 宋文质,.燃煤地区大气气溶胶烟炱的研究[J]. 环境化学, 1985, 4(专辑): 134-136.]

[25] Qin Shiguang,Tang Jie,Wen Yupu. Black carbon and its importance in climate change Studies[J]. Meteorology, 2001, 27(11):3-7.[秦世广,汤洁,温玉璞.黑碳气溶胶及其在气候变化研究中的意义[J]. 气象,2001,27(11):3-7.]

[26] Bodhaine B A. Aerosol absorption measurements at Barrow, Mauna Loa and the south pole[J]. Journal of Geophysical Research,1995, 100(D5): 8 967-8 975.

[27] Krivacsy Z, Hoffer A, Sarvari Zs, et al. Role of organic and black carbon in the chemical composition of atmospheric aerosol at European background sites[J]. Atmospheric Environment, 2001, 35: 6 231-6 244.

[28] Bizjak M, Turši?J, Lešnjak M, et al. Aerosol black carbon and ozone measurements at Mt. Krvavec EMEP/GAW station, Slovenia[J]. Atmospheric Environment, 1999, 33:2 783-2 787.

[29] Bhugwant C,Brémaud P. Simultaneous measurements of black carbon, PM10, ozone and NOx variability at a locally polluted island in the Southern Tropics[J]. Journal of Atmospheric Chemistry,2001, 39: 261-280.

[30] Bhugwant C, Cachier H, Bessafi M, et al. Impact of traffic on black carbon aerosol concentration at la Réunion Island (Southern Indian Ocean)[J]. Atmospheric Environment,2000, 34: 3 463-3 473.

[31] Chylek P, Videen D, Ngo R G, et al. Effect of black carbon on the optical properties and climate forcing of sulfate aerosol[J]. Journal of Geophysical Research, 1995, 100: 325-332.

[32] Cao J J, Lee S C, Ho K F, et al. Spatial and seasonal variations of atmospheric organic carbon and elemental carbon in Pearl River Delta Region, China[J]. Atmospheric Environment,2004,38:4 447-4 456.

[33] Li Yang, Cao Junji, Zhang Xiaoyi, et al. Variability of black carbon aerosol over Xi'an atmosphere[J]. The Chinese Journal of Process Engineering,2004,4(suppl.): 742-749.[李杨,曹军骥,张小曳,. 西安大气中黑碳气溶胶的演化特征[J]. 过程工程学报, 2004, 4(增刊): 742-749.]

[34] Zhang X Y, Wang Y Q, Wang D, et al. Characterization and sources of regional-scale transported carbonaceous and dust aerosols from different pathways in costal and sandy land areas of China[J]. Journal of Geophysical Research,2005, 110: D15301, doi:10.1029/2004JD005457.

[35] Im J-S, Saxena V K, Wenny B N. Temporal trends of black carbon concentrations and regional climate forcing in the southereastern United States[J]. Atmospheric Environment, 2001, 35: 3 293-3 302.

[36] Pakkanen T A, Kerminen V-M, Ojanen C H, et al. Atmospheric black carbon in Helsinki[J]. Atmospheric Environment, 2000, 34: 1 497-1 506.

[37] Castanho Andrea D A, Artaxo P. Wintertime and summertime São Paulo aerosol source apportionment study[J]. Atmospheric Environment,2001, 35: 4 889-4 902.

[38] Latha K M,Badarinath K V S. Black carbon aerosols over tropical urban environment—A case study[J]. Atmospheric Research,2003, 69: 125-133.

[39] Bizjak M, Cigler R, Hansen A D A, et al. Diurnal concentrations of black carbon and some other air pollutants in Ljubljana, Slovenia[J]. Atmospheric Environment,1993, 27A:1 347-1 350.

[40] Gatari M J,Boman J. Black carbon and total carbon measurements at urban and rural sites in Kenya, East Africa[J]. Atmospheric Environment,2003, 37: 1 149-1 154.

[41] Zhu Houling. The Study on the Temporal and Spatial Distribution of Black Carbon Aerosol in China[D]. Beijing: Chinese Academy of Meteorological Sciences,2003.[朱厚玲.我国地区黑碳气溶胶时空分布研究[D].北京:中国气象科学院,2003.]

[42] Hu Jianfang, Jia Guodong, Peng Ping'an, et al. Reconstruction of surface ocean water pCO2 (aq) in Nansha area, the South China Sea during the last 30 ka[J]. Chinese Science Bulletin, 2003, 48(2): 199-203.[胡建芳,贾国东,彭平安,.30ka来南沙海区表层水的PCO2记录[J].科学通报,2003,47(21):1 667-1 670.]

[43] Jia Guodong, Peng Ping'an, Sheng Guoying, et al. The sedimentary records of black carbon in Nansha sea area since the last glaciation[J]. Chinese Science Bulletin, 2000, 45(17): 1 594-1 596.[贾国东,彭平安,盛国英,.南沙海区末次冰期以来黑碳的沉积记录[J].科学通报,2000,45(6):646-650.]

[44] Martins J V, Artaxo P, Liousse C, et al. Effects of black carbon content, particle size, and mixing on light absorption by aerosols from biomass burning in Brazil[J]. Journal of Geophysical Research, 1998, 103(D24): 32 041-32 050.

[45] Reid J S, Hobbs P V, Liousse C, et al. Comparisons of techniques of measuring shorwave absorption and black carbon content of aerosols from biomass burning in Brazil[J]. Journal of Geophysical Research, 1998,103:32 031-32 040.

[46] Liousse C, Cachier H, Jennings S G. Optical and thermal measurements of black carbon aerosol content in different environments: Variation of the specific attenuation cross-section, sigma (s)[J]. Atmospheric Environment, 1993, 27A: 1 203-1 211.

[47] Babich P, Davey M, Allen G, et al. Method comparisons for particulate nitrate, elemental carbon, and PM2.5 mass in seven US cities[J]. Journal of Air and Waste Management Association, 2000, 50(7): 1 095-1 105.

[48] Hitzenberger R, Jennings S G, Larson S M, et al. Intercomparison of measurement methods for black carbon aerosols[J]. Atmospheric Environment,1999, 33:2 823-2 833.

 

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